[Blarg]

Two little girls?

Spirited Away is your #1 choice. A little girl is the main character. And it's a truly great movie.
All the other Miyazaki stuff.
Old Yeller.
Beauty and the Beast -- the original one in the 30s. Very magical and beautiful. I'm not sure if you can get it with voice-over instead of subtitles, though.
The Red Balloon.
King Kong
The Iron Giant
The Seven Voyages of Sinbad(I think that's the name -- old stop-motion Ray Harryhausen special effects, very fun)
Robin Hood, the original one
Frankenstein(original one, it's not scary, Franky is pretty lovable really)

All this stuff is decent to great for adults too.